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Electronic States of NdSb in Antiferromagnetism

This article examines the electronic structure of NdSb when it becomes antiferromagnetic.

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NdSb is a material that shows interesting electronic behaviors when cooled down to low temperatures. This article discusses what happens to its electronic structure, particularly in its surface states, when it transitions into an Antiferromagnetic state. Antiferromagnetism refers to a type of magnetism where adjacent magnetic moments point in opposite directions, resulting in no net magnetization.

Antiferromagnetic Properties

As NdSb cools below a certain temperature, it undergoes a magnetic phase transition, becoming antiferromagnetic. At this point, its internal magnetic order develops, leading to specific arrangements of magnetic moments across the material.

In the case of NdSb, three distinct types of Magnetic Domains can exist at the surface due to its antiferromagnetic characteristics. Understanding these domains helps shed light on how symmetry and Electronic States interact in materials.

Research Methodology

To study the electronic states of NdSb, angle-resolved photoemission spectroscopy (ARPES) was used. This technique allows researchers to analyze how electrons behave at the surface of the material when illuminated with focused light. By carefully directing the light and analyzing the resulting electron emissions, scientists can observe changes in the electronic states associated with the different magnetic domains.

Findings in the Paramagnetic Phase

In the paramagnetic phase, when NdSb is above the transition temperature, the electronic states appear relatively simple. The electronic structure is marked by various pockets in the so-called Fermi Surface, which corresponds to the energy levels that electrons can occupy.

These pockets are crucial in determining the overall behavior of the materials in electronic applications. The Fermi surface mapping during this phase indicates that NdSb does not exhibit significant complexity, and the electronic states are largely derived from bulk bands.

Transition to the Antiferromagnetic Phase

As the temperature drops below the transition point, NdSb enters the antiferromagnetic phase. This transition causes profound changes in the surface electronic states. The presence of multiple magnetic domains leads to varying arrangements of the magnetic moments at the surface.

Observations of Surface States

When researchers examined the surface electronic states in the antiferromagnetic phase, they identified unique patterns that depended on the type of magnetic domain present. Each domain exhibits a distinct symmetry, which influences the behavior of the surface states.

For example, in one of the magnetic domains, the surface states displayed a twofold symmetry around the edges of the bulk bands, while in another domain, a fourfold symmetric state was observed. These surface states are important because they can lead to enhanced electronic properties that are useful for various applications.

Understanding Symmetry and Surface States

The unique surface states observed are linked to how symmetry is broken at the surface of NdSb. When the material is in an antiferromagnetic state, the combination of surface effects and internal symmetry leads to new surface states that would not be present otherwise.

This interplay between symmetry and electronic states is essential for understanding the physical properties of NdSb and similar materials. The discovery of new surface states opens up pathways for research into their potential applications in advanced electronic devices.

The Role of Temperature

Temperature plays a critical role in shaping the electronic states of NdSb. As mentioned earlier, at high temperatures, the material exists in a simpler electronic state characterized by bulk-derived features. Upon cooling, certain bands appear, which are associated with the magnetically ordered state of the material.

The temperature dependence of these surface states reveals that they vanish when the material is heated above the transition temperature. This relationship highlights the strong link between the electronic structure and the magnetic behavior of the material.

Insights from Domain-Selective Studies

Using domain-selective measurements, researchers could differentiate between the electronic states corresponding to the different magnetic domains on the surface. By mapping out the electronic states selectively for each domain, it became evident that the surface states were a direct result of the unique arrangements of the magnetic moments.

For instance, in one domain, specific shallow bands were detected, which were related to the antiferromagnetic band folding. In contrast, another domain exhibited a simpler electronic structure without these additional surface features.

Implications of Surface States

The unique properties associated with the surface states of NdSb provide insights into potential applications in spintronics and quantum computing. The ability to manipulate surface states through control of magnetic ordering could lead to the development of materials with enhanced functional properties.

Moreover, the observed surface states also suggest that similar behaviors may be present in other antiferromagnetic materials. This could open new avenues in research aimed at discovering magnetic materials with tailored electronic properties.

Conclusion

The exploration of NdSb has revealed the fascinating relationship between magnetic order and electronic states. The identification of unusual surface states linked to antiferromagnetism highlights the complexity of condensed matter systems.

As we continue to uncover these relationships, a deeper understanding of how symmetry affects electronic properties will emerge, paving the way for innovative applications in advanced materials and devices. Further research is required to explore these findings and their implications in greater detail.

Original Source

Title: Unusual surface states associated with the PT-symmetry breaking and antiferromagnetic band folding in NdSb

Abstract: We have performed micro-focused angle-resolved photoemission spectroscopy on NdSb which exhibits the type-I antiferromagnetism below TN = 16 K. We succeeded in selectively observing the band structure for all three types of single-q antiferromagnetic (AF) domains at the surface. We found that two of the three surfaces whose AF-ordering vector lies within the surface plane commonly show twofold symmetric surface states (SSs) around the bulk-band edges, whereas the other surface with an out-of-plane AF-ordering vector displays fourfold symmetric shallow electronlike SS at the Brillouin-zone center. We suggest that these SSs commonly originate from the combination of the PT (space-inversion and time-reversal) symmetry breaking at the surface and the band folding due to the AF order. The present results pave a pathway toward understanding the relationship between the symmetry and the surface electronic states in antiferromagnets.

Authors: Asuka Honma, Daichi Takane, Seigo Souma, Yongjian Wang, Kosuke Nakayama, Miho Kitamura, Koji Horiba, Hiroshi Kumigashira, Takashi Takahashi, Yoichi Ando, Takafumi Sato

Last Update: 2023-09-13 00:00:00

Language: English

Source URL: https://arxiv.org/abs/2307.02878

Source PDF: https://arxiv.org/pdf/2307.02878

Licence: https://creativecommons.org/publicdomain/zero/1.0/

Changes: This summary was created with assistance from AI and may have inaccuracies. For accurate information, please refer to the original source documents linked here.

Thank you to arxiv for use of its open access interoperability.

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