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New Developments in Twisted Graphene Structures

Research reveals exciting properties of bulk alternating twisted graphite.

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In recent years, scientists have become very interested in twisted graphene structures. These are formed when two layers of graphene, which is a thin layer of carbon atoms arranged in a hexagonal pattern, are rotated relative to each other. This twisting creates a special pattern known as a moiré pattern, which can lead to unique and interesting behaviors in the material's electronic properties.

Twisted Bilayer Graphene (TBG) has gained particular attention because of the unique behaviors that arise when the twisting angle is near certain specific values, often called "Magic Angles." At these angles, the electronic bands in the material become very flat, which means that electrons in these bands behave differently compared to those in conventional materials. This has led to fascinating phenomena such as superconductivity and various quantum states.

Understanding the Twisted Graphene Spiral

Researchers have now developed a new type of material called the bulk alternating twisted graphite (ATG). This material consists of many layers of twisted graphene stacked on top of each other. The twist angle between these layers is held constant, resulting in a three-dimensional structure that has intriguing properties that differ from its two-dimensional counterparts.

The ATG is made using a chemical vapor deposition method, which allows for precise control over the twisting of the graphene layers. The additional dimension provided by stacking the layers gives scientists a new way to study the behavior of electrons in these materials.

Magic Momenta and Flat Bands

One of the key findings in this research is the concept of "magic momenta." In the bulk ATG, when the twist angle is smaller than twice the magic angle of TBG, there exist specific points in the material where the speed of electrons within certain bands becomes zero. These points are crucial for understanding the unique electronic behavior of the material, as they enable the coexistence of different electronic states that could lead to new physics.

When the twist angle is large, the material can exhibit a special type of Landau level, which is a quantized energy level of electrons in a magnetic field. Specifically, a dispersionless zeroth Landau level emerges, which may lead to strong Quantum Hall Effects across a wide range of twist angles.

The Role of Magic Angles

In TBG, when the twist angle is close to certain "magic angles," the electronic bands become flat, leading to strong correlations between electrons. This results in various exotic states of matter. The research indicates that the bulk ATG system can maintain these magic angles even as the twist angle varies, allowing for a rich set of electronic behaviors.

By stacking many layers of twisted graphene, researchers can introduce a new degree of freedom in tuning the electronic properties. This means they can explore how different angles and layer combinations affect the properties of the material.

The Growth of Twisted Graphene Structures

Using an origami-like approach, scientists have managed to grow a spiral structure made of multiple layers of twisted graphene. This double-helix configuration is achieved through careful control during the growth process, allowing for layers of graphene to be twisted in a uniform manner.

This spiraling structure enhances the interactions between the graphene layers, leading to new types of moiré patterns and electronic behaviors. The growth technique also provides a pathway for creating materials with tailored properties for specific applications.

Observing Unique Electronic Properties

The electronic structure of the bulk ATG system has shown that it can host multiple flat bands that arise from TBG at different magic angles. This means that by adjusting the twist angle, a broad range of electronic states can coexist, paving the way for unprecedented phases of matter.

The research also indicates strong topological properties within the ATG, where the introduction of small mass terms can lead to changes in the material's electronic characteristics. These topological states can be manipulated, leading to new phenomena and insights.

Landau Levels in the Bulk ATG

The study of Landau levels is essential for understanding the behavior of electrons in a magnetic field. In the bulk ATG, a chain of these Landau levels aligns in a way that is unique to the three-dimensional structure. These Landau levels can exhibit different behaviors depending on the twist angle and external conditions such as magnetic fields.

With a strong magnetic field applied, the zeroth Landau level remains pinned at a specific energy, which leads to a stable electronic state in the material. This robustness against disorder and inhomogeneity is a significant feature of the ATG.

Quantum Hall Effects in Three Dimensions

The unique band structure of the bulk ATG suggests that it can exhibit three-dimensional quantum Hall effects. Unlike traditional two-dimensional systems, where quantum Hall effects are typically observed, the three-dimensional nature allows for even more complex interactions between electrons.

When certain Landau levels are occupied, robust quantized conductivities are expected, which can lead to interesting phase transitions and exotic states of matter. These behaviors may find applications in various fields, including quantum computing and advanced electronic devices.

Conclusion and Future Directions

The ongoing research into twisted graphene structures like bulk ATG promises to uncover new physics beyond what is currently understood. As scientists continue to investigate these materials, it is expected that they will discover new phenomena and applications in technology.

By exploring the effects of multiple layers, varying twist angles, and external conditions, researchers can significantly expand the understanding of two-dimensional materials and their behaviors in three dimensions. This work lays the groundwork for future studies that could lead to groundbreaking advancements in materials science.

Original Source

Title: Magic momenta and three dimensional Landau levels from a three dimensional graphite moir\'e superlattice

Abstract: Twisted bilayer graphene (TBG) and other quasi-two-dimensional moir\'e superlattices have attracted significant attention due to the emergence of various correlated and topological states associated with the flat bands in these systems. In this work, we theoretically explore the physical properties of a new type of \textit{three dimensional graphite moir\'e superlattice}, the bulk alternating twisted graphite (ATG) system with homogeneous twist angle, which is grown by in situ chemical vapor decomposition method. Compared to TBG, the bulk ATG system is bestowed with an additional wavevector degrees of freedom due to the extra dimensionality. As a result, we find that when the twist angle of bulk ATG is smaller than twice of the magic angle of TBG, there always exist ``magic momenta" at which the in-plane Fermi velocities of the moir\'e bands vanish. Moreover, topologically distinct flat bands of TBG at different magic angles can even co-exist at different out-of-plane wavevectors in a single bulk ATG system. Most saliently, when the twist angle is relatively large, exactly dispersionless three dimensional zeroth Landau level would emerge in the bulk ATG, which may give rise to robust three dimensional quantum Hall effects over a large range of twist angles.

Authors: Xin Lu, Bo Xie, Yue Yang, Xiao Kong, Jun Li, Feng Ding, Zhu-Jun Wang, Jianpeng Liu

Last Update: 2023-09-02 00:00:00

Language: English

Source URL: https://arxiv.org/abs/2309.00825

Source PDF: https://arxiv.org/pdf/2309.00825

Licence: https://creativecommons.org/licenses/by/4.0/

Changes: This summary was created with assistance from AI and may have inaccuracies. For accurate information, please refer to the original source documents linked here.

Thank you to arxiv for use of its open access interoperability.

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