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Chirality in Magnetic Materials and DMI

Investigating the role of chirality and DMI in magnetic materials' behavior.

― 5 min read


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Chirality is a property that can be found in many natural objects, such as DNA and some sugars. In magnetism, it refers to the way certain magnetic patterns behave when there is a lack of symmetry. This is especially seen in systems where a unique type of magnetic interaction, known as the Dzyaloshinskii-Moriya Interaction (DMI), occurs. This interaction leads to the formation of twisted magnetic structures.

The Dzyaloshinskii-Moriya Interaction

DMI arises in materials that have broken inversion symmetry, meaning their structure is not the same when mirrored. It involves spins, which are tiny magnetic moments found in materials. The DMI can cause these spins to align in a manner that creates a twist, resulting in chiral magnetic textures. This behavior can be affected by the arrangement and type of atoms in the magnetic material.

Experimental Approach

To investigate how chirality in magnetic materials works, researchers have created special layered structures. These structures are made by stacking alternating layers of Ferromagnetic Metals on a surface known as Ir(001). By analyzing these layered systems, researchers aim to understand how the DMI behaves at a very small, atomic scale.

One key observation is that the DMI's strength and direction rely heavily on the type of atoms at the interface and how the atomic layers are stacked. As the number of layers increases, the interactions become more complex, leading to a variety of magnetic behaviors.

Role of Atomic Layers

When ferromagnetic metals like iron (Fe), cobalt (Co), and nickel (Ni) are deposited on a substrate with strong spin-orbit coupling like Ir(001), the DMI can lead to the formation of chiral spin patterns. The arrangement of these atomic layers plays a crucial role in determining the DMI's effectiveness.

Researchers have discovered that the characteristics of the DMI change depending on two main factors. The first is the number of Unpaired Electrons in the atomic layers that are closest to the substrate. The second is how these atomic layers are arranged. Each layer contributes to the overall magnetic interactions, and changing their order can impact the DMI's strength and chirality.

Experimenting with Different Layer Combinations

In their studies, researchers created various combinations of atomic layers, such as double and triple layers of Fe, Co, and Ni on the Ir(001) substrate. Each combination affects the DMI in unique ways. The goal is to determine how the number and sequence of layers influence the DMI's properties.

As they conduct experiments, it becomes evident that the number of unpaired electrons in the interface layer is a major factor for both the strength and the chirality of the DMI. For example, having a high number of unpaired electrons typically increases the DMI's strength.

Measuring the DMI

To measure the effects of DMI in these experiments, researchers use a technique called spin-polarized high-resolution electron energy loss spectroscopy (SPHREELS). This method allows scientists to probe the energy and behavior of collective magnetic excitations, which are essential for understanding the DMI.

By studying how the energy of these excitations changes in different magnetic environments, researchers can gather valuable insights into the nature of DMI and its dependence on the arrangement of atomic layers.

Observing Patterns

Researchers observe that as they change the sequence and number of atomic layers, the DMI behaves differently. For instance, the DMI is often stronger at the interface of Fe and Ir than at the interface of Co and Ni. Each material's unique electronic structure-how its electrons are arranged-plays a crucial role in these interactions.

The results show a complex relationship between the number of unpaired electrons and the overall behavior of the DMI. In some cases, an increase in unpaired electrons does not straightforwardly lead to a larger DMI, indicating the influence of the intricate patterns present in the atomic layers.

Complexity of Interactions

With increasing complexity in materials, the predictions about how the DMI behaves become less clear. The arrangement of atoms and their electronic properties creates a situation where the interactions are not easily linear or predictable.

Researchers find that the behavior of the DMI can change significantly based on the type and sequence of the atomic layers. By understanding these interactions better, they hope to find ways to control the DMI effectively, which could lead to new applications in magnetic devices.

Importance of Electronic Structure

The electronic structure, which describes how electrons are distributed in a material, is foundational to understanding the DMI. The interactions that lead to chirality hinge on how these electrons overlap and form hybrid states. Changing the composition of the atomic layers affects this electronic structure, and, consequently, influences the DMI.

In essence, these interactions control the way magnetic materials behave on an atomic level, and a deeper understanding could pave the way for advancements in technology, such as in data storage and processing.

Future Directions

As research continues, it becomes clear that optimizing the DMI by adjusting atomic layer configurations opens new pathways for engineering magnetic materials. The insights gained from studying these layered structures may lead to better ways to tune and utilize DMI for practical applications.

One promising area is in the development of new materials for spintronics, where the spin of electrons, as well as their charge, is used for information processing. Understanding and controlling DMI could lead to faster and more efficient devices.

Conclusion

Chirality in magnetic materials, driven by the Dzyaloshinskii-Moriya interaction, is a complex phenomenon that offers a glimpse into the future of magnetic technology. By studying the intricate relationships between atomic layers and their electronic properties, researchers aim to harness the unique behaviors of these materials for practical applications. The ongoing research promises exciting developments in magnetism and materials science, with potential impacts across various fields.

Original Source

Title: Unraveling the complexity of the Dzyaloshinskii-Moriya interaction in layered magnets: Towards its full magnitude and chirality control

Abstract: Chirality is an inherent characteristics of some objects in nature. In magnetism chiral magnetic textures can be formed in systems with broken inversion symmetry and due to an antisymmetric magnetic interaction, known as Dzyaloshinskii--Moriya interaction (DMI). Here, aiming on a fundamental understanding of this chiral interaction on the atomic scale, we design several synthetic layered structures composed of alternating atomic layers of 3d ferromagnetic metals epitaxially grown on Ir(001). We demonstrate both experimentally and theoretically that the atomistic DMI depends critically not only on the orbital occupancy of the interface magnetic layer but also on the sequence of the atomic layers. The effect is attributed to the complexity of the electronic structure and the contribution of different orbitals to the hybridization and DMI. We anticipate that our results provide guidelines for controlling both the chirality and the magnitude of the atomistic DMI.

Authors: Khalil Zakeri, Albrecht von Faber, Sergiy Mankovsky, Hubert Ebert

Last Update: 2024-02-28 00:00:00

Language: English

Source URL: https://arxiv.org/abs/2402.18466

Source PDF: https://arxiv.org/pdf/2402.18466

Licence: https://creativecommons.org/licenses/by/4.0/

Changes: This summary was created with assistance from AI and may have inaccuracies. For accurate information, please refer to the original source documents linked here.

Thank you to arxiv for use of its open access interoperability.

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