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# Physics# Strongly Correlated Electrons# Superconductivity

Investigating Light-Matter Interactions with Ultrafast Lasers

Research explores ultrafast laser pulses on metals and superconductors.

Kazuya Shinjo, Shigetoshi Sota, Seiji Yunoki, Takami Tohyama

― 6 min read


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In the world of physics, the interaction of light and matter can lead to some pretty fascinating outcomes. One of the hottest topics these days revolves around what happens when you hit materials like metals or superconductors with very short bursts of laser light. Picture a tiny flash that’s so brief it lasts less time than a blink. This kind of experimentation can help us figure out exciting features of these materials.

What Are Ultrafast Laser Pulses?

Ultrafast laser pulses are exactly what they sound like. They are bursts of laser light that last a very short time-often just a fraction of a billionth of a second. These laser pulses are used to probe materials and observe how they behave when excited by light. Just as you might react differently if someone surprises you with a sudden loud noise, materials can behave in wildly different ways when hit with these tiny flashes of light.

The Basics: Metallic and Superconducting States

Let’s break a few things down. Metals are materials that can conduct electricity well, meaning electrons move through them easily. Superconductors, on the other hand, can conduct electricity with zero resistance when cooled to very low temperatures. This means they can carry electrical current without any energy loss-a bit like a magic highway for electricity!

The Magic of Halfcycle Pulses

Now, imagine you had a special type of pulse-a halfcycle pulse. Instead of going through a whole cycle like a regular wave, it only goes halfway. This tiny twist can unlock unique states in the material being hit. A halfcycle pulse can create conditions that regular pulses fail to reach, leading to intriguing behaviors in electrons.

Pump-probe Spectroscopy: A Fancy Way to Look Under the Hood

To study how materials respond to these ultrafast pulses, scientists use a technique called pump-probe spectroscopy. It’s a bit like taking a quick peek under the hood of a car to see how the engine is running.

In this setup, the "pump" pulse does the excitation (the surprise) and a "probe" pulse follows up to see what’s changed afterward. By measuring the response of the material over time, researchers can learn a lot about how it works.

The Hubbard Model: A Framework for Understanding

To make sense of all the buzzing activity happening in these materials, scientists often use a theoretical model called the Hubbard model. This is a fancy tool that helps to describe how electrons behave in different situations. It’s often used to explore complex issues in physics, especially in strongly correlated systems (where the actions of electrons are closely tied to one another).

What Happens in Superconductors?

When a halfcycle pulse hits a superconductor, something interesting happens. This pulse can activate what are known as amplitude modes. These modes are related to the way the Superconducting Pairs of electrons behave. It’s like giving the electrons a little nudge and watching how they dance together.

In some cases, this nudge can lead to a measurable change in optical absorption, which is a way of saying that the material is absorbing light at certain energies. Scientists have found these absorptions at energies that correspond to what’s called the Higgs mode-the fancy dance of electrons in a superconductor.

What About Metals?

Metals react differently when hit with a halfcycle pulse. Instead of the focused dance of superconducting electrons, the pulse causes a broader range of absorptions. These absorptions can spread across various energy levels, especially those associated with magnetic excitations. It’s a bit like throwing a handful of confetti into the air and watching how each piece behaves.

The Experiment: What Researchers Did

In their quest for knowledge, researchers decided to study both one-dimensional (1D) and two-dimensional (2D) Hubbard Models using this halfcycle pulse technique. Picture them playing with theoretical toy models to see how the electrons would behave.

They set up experiments to simulate how these materials would react and measure their Absorption Spectra, the fancy term for how much light gets absorbed at different energies. This is like having a special camera that can capture how much light gets eaten up by different parts of the material.

Findings: Superconductors vs. Metals

When studying superconductors, the experiments showed that the absorption patterns were closely tied to the Higgs mode that we talked about earlier. The response was sharp, indicating a clear relationship between the supercurrent (the flow of electricity) and the absorption of light.

In contrast, for metals, the results were more diffuse, indicating a broader range of energy absorption. The different types of absorptions revealed that the excited states are more complex in metals compared to superconductors.

The Power of Disorder

Now, let’s add a twist-disorder! In real life, materials are rarely perfect. They often have defects or impurities that can change their behavior. In superconductors, introducing disorder can lead to changes in how absorptions occur. Even if a superconductor is clean, the presence of supercurrents can still affect how it absorbs light, shifting the patterns of absorption significantly.

Why Is This Important?

Understanding these interactions is more than just a game for physicists. It has real-world implications for developing new technologies. Superconductors, for example, have applications in everything from advanced computing to powerful magnets used in MRI machines. By mastering how light interacts with these materials, we can help build better, more efficient systems.

Future Directions: What’s Next?

So, what’s next in the world of ultrafast laser pulses and material science? Researchers are looking into larger systems and advanced techniques to gain even deeper insights. They want to understand the nuances between different types of superconductors and metals and how their unique interactions could lead to new discoveries.

Moreover, as technology progresses, it may be possible to create tailored materials that can respond more effectively under certain conditions. Scientists are excited about the potential of this research and what it might lead to in the future.

Conclusion: Light Unleashing New Possibilities

In the grand dance of particles and waves, ultrafast laser pulses are like surprise guest stars, stepping into the spotlight and changing how the show unfolds. Whether teasing out the secrets of superconductors or revealing the mysteries of metals, these research efforts are setting the stage for future innovations and discoveries. So, the next time you think about light, remember-it’s not just about illumination; it’s also about unlocking the hidden properties of materials in the blink of an eye.

Original Source

Title: Optical absorptions activated by an ultrashort halfcycle pulse in metallic and superconducting states of the Hubbard model

Abstract: The development of high-intensity ultrashort laser pulses unlocks the potential of pump-probe spectroscopy in sub-femtosecond timescale. Notably, subcycle pump pulses can generate electronic states unreachable by conventional multicycle pulses, leading to a phenomenon that we refer to as subcycle-pulse engineering. In this study, we employ the time-dependent density-matrix renormalization group method to unveil the transient absorption spectra of superconducting and metallic states in nearly half-filled one-dimensional and two-dimensional Hubbard models excited by an ultrashort halfcycle pulse, which can induce a current with inversion-symmetry breaking. In a superconducting state realized in attractive on-site interactions, we find the transient activation of absorptions at energies corresponding to the amplitude modes of superconducting and charge-density-wave states. On the other hand, in a metallic state realized in the two-dimensional model with repulsive on-site interactions, we obtain another type of absorption enhancements, which are distributed broadly in spin excitation energies. These findings indicate that superconducting and metallic states are sensitive to an ultrashort halfcycle pulse, leading to the transient activations of optical absorptions with their respective mechanisms.

Authors: Kazuya Shinjo, Shigetoshi Sota, Seiji Yunoki, Takami Tohyama

Last Update: 2024-10-31 00:00:00

Language: English

Source URL: https://arxiv.org/abs/2411.00313

Source PDF: https://arxiv.org/pdf/2411.00313

Licence: https://creativecommons.org/licenses/by/4.0/

Changes: This summary was created with assistance from AI and may have inaccuracies. For accurate information, please refer to the original source documents linked here.

Thank you to arxiv for use of its open access interoperability.

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